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I am set up in The Castle. I have shops set up in the interior. Armory/mess hall stuff in the courtyard. Houses on the walls.
There is not a ton of settlements nearby that you can enslave, but its such a fun place to defend from attacks.
Comes down to what I am playing as. If I am a minuteman then Sanctuary and once I can Bunker Hill. If I am a raider, Starlight then the build I made for The Castle. If I am a BOS then the Airport. If I am playing as someone from the institute then my house in DC.